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A suspension consisting of particles (grey) dispersed in a fluid (dark blue) is (a) placed onto a freezing substrate; (b) solid dendrites (light blue) propagate in the direction of the thermal gradient while pushing particles away from the moving front.1.. IntroductionTape casting is an established method for manufacturing wide and flat sheets of ceramic materials. Most applications of tape casting technology refer to the electronic industry, while some authors have also used this technique for obtaining thin ceramic sheets and multilayered structures for different application such as solid oxide fuel cells or laminated composites. 1, 2, 3 ...Titanium dioxide (TiO2) is one of the most widely used materials in resistive switching applications, including random-access memory, neuromorphic computing, biohybrid interfaces, and sensors. Most of these applications are still at an early stage of development and have technological challenges and a lack of fundamental comprehension. 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